Joint Workshop LANL/NIMS Quantum and Functional Materials and MANA International Symposium 2024


Session 6-1

Title

Quantum Emitters in Flatland

Author's photo

Authors

Han Htoon

Affiliations

Center for Integrated Nanotechnologies, Los Alamos National Laboratory

URL

https://lanlexperts.elsevierpure.com/en/persons/han-htoon

Email

htoon@lanl.gov

Abstract

In this talk, I will highlight our recent efforts on the development of new class of 2D material-based quantum light emitters and exploit of proximity interactions in realization of chiral quantum light emitters. 2D-Quantum emitters have generated a lot of excitement for their potential in quantum information technologies. Most of the QE realized to date operate at wavelengths shorter than 1 micron. Here I will present three new 2D quantum emitters capable of wavelength tunable single photon emission across 1000-1600 nm NIR spectral range and operation at liquid nitrogen temperatures. The QEs were realize via strain engineering of MoTe2,[1] WSe2/MoS2,[2] and InSe2[3] 2D materials.
Next, I will show that circularly polarized single photon emission can be achieved without the application of a high external magnetic field, injection of spin-polarized carriers and coupling to complex chiral metamaterial structures. Our experiment shows that QE created at the same location as the magnetic defect in 2D correlated antiferromagnet, NiPS3, can borrow magnetic properties of the magnetic defect through proximity induced exchange interaction and emit circularly polarized single photons.[4]

Fig. 1. Strain engineering of 2D TMD layer via use of nanopillar array leads to formation of quantum light emitters
Fig. 2. Chiral quantum light emitters are created by nano indentations of WSe2/NiPS3, TMD/2D antiferromagnetic heterostructure .

Reference

  1. Zhao, H., Pettes, M. T., Zheng, Y. & Htoon, Nature Communications 12, 1-7 (2021). DOI:10.1038/s41467-021-27033-w
  2. Zhao, H., et al., Nano Letters 23, 11006-11012 (2023). DOI: 10.1021/acs.nanolett.3c03296
  3. Zhao, H. et al., Telecom-wavelength Single-photon Emitters in Multi-layer InSe. Submitted to ACS Nano. (2024).