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Poster QM-13

Spin Transport Phenomena in Janus Transition Metal Dichalcogenides

Tomoaki Kameda

Author

Tomoaki Kameda, Souren Adhikary, Katsunori Wakabayashi

Affiliation

Quantum Materials Design Group, MANA, NIMS

URL

https://www.kg-nanotech.jp/tmd/

Biography

Tomoaki Kameda is a Ph.D. student at Kwansei Gakuin University and a Junior Researcher at the National Institute for Materials Science (NIMS), Japan. His research focuses on theoretical condensed matter physics and electronic transport in two-dimensional materials. His current research focuses on spin-current generation and nonlinear transport phenomena in Janus transition-metal dichalcogenides.

Abstract

Two-dimensional transition metal dichalcogenides (TMDCs) provide a versatile platform for controlling spin and charge transport through crystal-symmetry engineering and spin–orbit coupling (SOC) [1]. In Janus TMDCs [2], inequivalent top and bottom chalcogen layers break the out-of-plane mirror symmetry and generate an internal electric field, leading to Rashba-type SOC. Here, we theoretically investigate linear spin and nonlinear charge transport in Janus TMDCs. For monolayer 1H-WSeTe, a tight-binding model shows that linearly polarized light can generate pure spin Hall currents (Fig. 1), and Rashba SOC plays a key role in determining the spin-polarization direction and enhancing the spin-current response [3]. We further study nonlinear transport in 1T′-Janus TMDCs (Fig. 2). While crystal symmetries suppress the Berry-curvature dipole in pristine systems, Janus-induced symmetry breaking allows a finite Berry-curvature dipole, resulting in a nonlinear Hall charge current without external strain. These results demonstrate that Janus engineering provides a route to control distinct spin and charge responses through symmetry breaking and band geometry, offering design principles for low-dimensional spintronic and nonlinear electronic devices.

Spin Hall current and spin-dependent optical conductivity in Janus TMDCs
Fig. 1. (a) Schematic of the generation of spin Hall currents under the linearly polarized light irradiation. (b) Spin-dependent optical conductivity in Janus TMDCs, with photon incidence along the y-direction and conductivity measured along the x-direction. The spin polarization is along the y-direction. The red (black) line represents the conductivity with (without) Rashba SOC.
Top and side views of monolayer 1T′-Janus TMDCs
Fig. 2. (a) Top view of monolayer 1T’-Janus TMDCs, illustrating the 1st nearest-neighbor, 2nd nearest-neighbor, 3rd nearest-neighbor, 4th nearest-neighbor, 5th nearest-neighbor and 6th nearest-neighbor hopping vectors. (b) Side view of monolayer 1T’-Janus TMDCs, showing the transition metal layer sandwiched between two different chalcogen layers, labeled as Chalcogen 1 and Chalcogen 2.

References

  1. S. Manzeli and A. Kis. et.al. Nat. Rev. Mater. 2, 17033 (2017). DOI: 10.1038/natrevmats.2017.33
  2. J. Zhang et al. ACS Nano 11, 8192–8198 (2017). DOI: 10.1021/acsnano.7b03186
  3. T. Kameda, K. Wakabayashi, Phys. Rev. B 111, 195425 (2025). DOI: 10.1103/PhysRevB.111.195425
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MANA
JSPS
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